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Abstrak :
[Gas alam sudah menjadi alternatif bahan bakar maupun digunakan sebagai bahan baku industri. Gas alam terdiri dari senyawa hidrokarbon berupa gas, seperti metana, etana, propana, butana, dan kondensat. Namun gas alam memiliki kandungan pengotor berupa air, nitrogen, karbon dioksida, hidrogen sulfida, dan merkuri yang harus dihilangkan. Teknologi kontaktor membran merupakan salah satu cara dalam menghilangkan kandungan karbon dioksida yang terdapat di dalam gas alam. Pada penelitian ini digunakan teknologi kontaktor membran serat berongga superhidrofobik dengan menggunakan pelarut DEA. Penelitian ini bertujuan untuk mengetahui persen penyerapan gas karbon dioksida dari pelarut DEA serta untuk mengetahui pengaruh laju alir gas umpan terhadap fenomena perpindahan massa yang terjadi di membran. Dari fenomena perpindahan massa yang terjadi, akan didapatkan kinerja dari kontaktor membran serat berongga superhidrofobik dalam proses absorbsi gas karbon dioksida. Berdasarkan penelitian yang dilakukan, jumlah gas karbon dioksida yang terserap sebesar 0,03128-0,05331 mmol/s untuk modul dengan jumlah serat 8000 dan untuk modul dengan jumlah serat 2000 mampu menyerap gas CO2 sebesar 0,0268-0,02994 mmol/s. Nilai koefisien perpindahan massa yang didapatkan untuk modul dengan jumlah serat 2000 adalah sebesar 1,93x10-4-2,5x10-4 cm/s dan modul dengan jumlah serat 8000 sebesar 9,8x10-5 – 1,44x10-4 cm/s untuk variasi laju alir gas sebesar 170, 255, dan 340 cm3/min dengan laju alir pelarut DEA yang tetap sebesar 500 cm3/min. ......Natural gas has been used as alternative fuel or used as industrial raw materials. Natural gas consists of hydrocarbon compounds such as methane, ethane, propane, butane, dan condensats. However, natural gas also consists of impurities such as water, nitrogen, carbon dioxide, hydrogen sulfide, and mercury which have to remove. Membrane contactor technology is one of the methods which is used to remove carbon dioxide contents that contained in natural gas. In this study, we use hollow fiber membrane contactor using DEA as the solvent. The aim of this study is to know the absorption percentage of carbon dioxide and to know the effect of feed gas flow to mass transfer phenomenon which is occurred in membrane contactor. From the mass transfer phenomenon, we will obtain the performance of superhydrophobic hollow fiber membrane contactor in the absorption process. According to this study, the amount of carbon dioxide absorbed are about 0,03128-0,05331 mmol/s for the module with 8000 fibers and for the module with 2000 fibers able to absorb CO2 about 0,0268-0,02994 mmol/s. The value of mass transfer coefficient which yang is obtained from the module with 2000 fibers are 1,93x10-4-2,5x10-4 cm/s and for the module with 8000 fibers are 9,8x10-5-1,44x10-4 cm/s for the variation of the feed gas flow: 170, 255, dan 340 cm3/min with the DEA constant flowrate about 500 cm3/min., Natural gas has been used as alternative fuel or used as industrial raw materials. Natural gas consists of hydrocarbon compounds such as methane, ethane, propane, butane, dan condensats. However, natural gas also consists of impurities such as water, nitrogen, carbon dioxide, hydrogen sulfide, and mercury which have to remove. Membrane contactor technology is one of the methods which is used to remove carbon dioxide contents that contained in natural gas. In this study, we use hollow fiber membrane contactor using DEA as the solvent. The aim of this study is to know the absorption percentage of carbon dioxide and to know the effect of feed gas flow to mass transfer phenomenon which is occurred in membrane contactor. From the mass transfer phenomenon, we will obtain the performance of superhydrophobic hollow fiber membrane contactor in the absorption process. According to this study, the amount of carbon dioxide absorbed are about 0,03128 – 0,05331 mmol/s for the module with 8000 fibers and for the module with 2000 fibers able to absorb CO2 about 0,0268 – 0,02994 mmol/s. The value of mass transfer coefficient which yang is obtained from the module with 2000 fibers are 1,93x10-4 – 2,5x10-4 cm/s and for the module with 8000 fibers are 9,8x10-5 – 1,44x10-4 cm/s for the variation of the feed gas flow: 170, 255, dan 340 cm3/min with the DEA constant flowrate about 500 cm3/min.]

Abstrak :
Pemisahan gas CO2/N2 memiliki peran yang vital dalam berbagai industri yang memiliki proses pembakaran. Teknologi alternatif untuk proses tersebut ialah kontaktor membran serat berongga karena dapat mengatasi kelemahan pada kolom konvensional, meskipun masih dapat terjadi pembasahan membran oleh pelarut. Oleh karena itu, penelitian ini akan menguji pengaruh konsentrasi dan laju alir pelarut serta jumlah serat membran pada kinerja penyerapan CO2 melalui kontaktor membran serat berongga superhidrofobik. Pelarut yang digunakan yaitu polietilena glikol PEG. Variasi konsentrasi yaitu 5, 10, 15, dan 20 -b/v. Variasi laju alir pelarut yaitu 100, 200, 300, 400, dan 500 cm3/menit. Variasi jumlah serat membran yaitu 1000, 3000, dan 5000. Setiap percobaan dilakukan pada laju alir gas 190 SCCM. Pada uji hidrodinamika, penurunan tekanan maksimal di dalam serat membran yaitu 24,8 kPa dan rasio penurunan tekanan maksimal yaitu 1,69. Konsentrasi pelarut yang optimum yaitu pada rentang 5-10 -b/v untuk kondisi operasi yang digunakan. Parameter kinerja perpindahan massa maksimal yang diperoleh antara lain koefisien perpindahan massa 5,85x10-7 m/s, fluks perpindahan massa 2,11x10-5 mol/m2.s, CO2 loading 9,96x10-3 mol CO2/mol PEG, efisiensi penyerapan 33,27 , dan jumlah CO2 terabsorpsi 5,65x10-6 mol/s. ......The separation of CO2 N2 has a vital role in nowadays industries which have combustion process. The alternative technology for that process is hollow fiber membrane contactor because it is able to overcome the disadvantages of conventional column, although there is still wetting phenomenon by the solvent. Therefore, this study will evaluate the effect of solvent concentration and flow rate and also the number of fibers in CO2 absorption performance through superhydrofobic hollow fiber membrane contactor. The abosrbent used is polyethylene glycol PEG. The solvent concentration variation are 5, 10, 15, and 20 w v. The solvent flow rate variation are 100, 200, 300, 400, and 500 mL minute. The number of fibers variation are 1000, 3000, and 5000. Each experiments are being done with gas flow rate of 190 SCCM. At hydrodynamic test, the maximal pressure drop in the fiber is 24,8 kPa and the maximal pressure drop ratio is 1,69. The optimum range for solvent concentration is 5 10 w v for the selected operating condition. Maximal mass transfer parameters calculated are 5,85x10 7 m/s for mass transfer coefficient, 2,11x10 5 mol m2.s for mass transfer flux, 9,96x10 3 mol CO2 mol PEG for CO2 loading, 33,27, for absorption efficiency, and 5,65x10 6 mol s for amount of absorbed CO2.